Throughout most of her career, Carole Laure primarily collaborated with Anglophone singer, songwriter, producer, and director Lewis Furey, whom she met in 1977 and who later became her husband. She debuted as a singer on the album Alibis in 1978.
In 1989, she devoted an acoustic-oriented bilingual album, Western Shadows, to country and western standards. The album featured cover versions of Tammy Wynette's "Stand By Your Man", Phil Spector's "To Know Him is to Love Him", Roseanne Cash's "Seven Ye